Rosenfeld functional for non-additive hard spheres

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LETTER TO THE EDITOR Rosenfeld functional for non-additive hard spheres

The fundamental measure density functional theory for hard spheres is generalized to binary mixtures of arbitrary positive and moderate negative nonadditivity between unlike components. In bulk the theory predicts fluid-fluid phase separation into phases with different chemical compositions. The location of the accompanying critical point agrees well with previous results from simulations over ...

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ژورنال

عنوان ژورنال: Journal of Physics: Condensed Matter

سال: 2004

ISSN: 0953-8984,1361-648X

DOI: 10.1088/0953-8984/16/30/l01